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XUV lasing during strong-field assisted transient absorption in molecules

机译:XUV激光在强场辅助瞬态吸收过程中   分子

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摘要

Using ab-initio non-Born-Oppenheimer simulations, we demonstrateamplification of XUV radiation in a high-harmonic generation type process usingthe example of the hydrogen molecular ion. A small fraction of the molecules ispumped to a dissociative Rydberg state from which IR-assisted XUV amplificationis observed. We show that starting at sufficiently high IR driving fieldintensities the ground state molecules become quasi-transparent for XUVradiation, while due to stabilization gain from Rydberg states is maintained,thus leading to lasing from strongly driven Rydberg states. Further increase ofthe IR intensity even leads to gain by initially unexcited molecules, which arequickly excited by the driving IR pulse.
机译:使用从头开始的非Born-Oppenheimer模拟,我们以氢分子离子为例,演示了高谐波产生型过程中XUV辐射的放大。一小部分分子被泵送至解离的Rydberg状态,从中可以观察到IR辅助XUV扩增。我们表明,从足够高的红外驱动场强开始,基态分子对XUV辐射变为准透明,而由于保持了里德堡态的稳定增益,因此导致了强驱动里德堡态的发射。 IR强度的进一步增加甚至会导致最初未被激励的分子获得增益,这些分子最初被驱动IR脉冲激发。

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